Pokemon Ruby Sapphire and Emerald
Pokemon HeartGold and SoulSilver

Why can't certain Pokemon learn the Surf move?



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I'm not sure what you mean, but generally if a Pokemon can't learn Surf, it means they just aren't the right species. For example, a Vaporeon could learn Surf, but a Rattata couldn't. It doesn't matter how many Pokemon or what items you're carrying. Some Pokemon just will never be able to learn certain moves - like Surf.