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Pounds are weight and cups are volume (size). They are not convertible to each other unless you know the density of the substance being measured.
However, assuming that Crisco is a brand of shortening in this case, then the manufacturer says 1 teaspoon weighs 12 grams.
1 cup [US] = 48 Teaspoon [US]
so one cup [US] = 48*12 = 576 grams
1 gram = 0.00220462 pounds
576 grams = 576 * 0.00220462 = 1.26986112 pounds
So a pound of Crisco will measure less than a cup.
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