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The Top of His Head - soundtrack - was created in 1989.
Yes, their song "Head Above Water" is on the Transformers 3 soundtrack.
All I can think of off the top of my head is "Follow the Leader" by Eric B and Rakim
The soundtrack that has the song Relax on it is the Zoolander Soundtrack. The song was performed by Frankie Goes to Hollywood.
It is on the Avatar soundtrack.