I looked despairingly at your question and wondered how someone couldn't look that up on their own.
"Why can't you understand?," she asked despairingly Source: http://www.thefreedictionary.com/despairingly
I despairingly entered my question at WikiAnswers for help with finding a sentence containing the word 'despairingly' because I was SO desperate that I forgot that the dictionary may well have a good example right there with the word's definition. Her sigh was despairingly disturbing.
Some synonyms for desperately are urgently or despairingly.
The likely word is "despairingly" (hopelessly, worriedly).
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