Answer 1
It is a matter of personal opinion. We don't know you, so we don't know what your preferences are. There are opinions below:
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Opinion 1
Some of my personal favorites are Busou Renkin, Gurren Lagann, and Fushigi Yuugi. However, I know nothing about what kind of anime you are into you may not like them.
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Opinion 2
hitman reborn and bleach
you can watch kamichama karin
Gogoanime.com is good
I highly recommend mumonkey websiteAnivide.com and luffymonkey.com are both good to watch anime on, however some of the series they have are dubbed, and some are subbed.
I think Yu Yu Hakusho is a good anime to watch.
mar. the fighting is more magic
Anime Season
FullMetal Alchemist .
MySpace are some other things besides Crunchyroll to watch anime on.
animefreak
highschool dxd has good story but not neccesarily a.....
Anime and Manga: Gakuen Mokushiroku: High School Of The Dead
You should watch Vamprire Knight, it was on of my first animes and it was epic ^_^ Its really good for subs