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Ideally, the Master Ball is what you want to catch Latios/Latias, because their legendary status makes them difficult to catch. If not the Master Ball, I recommend the Timer Ball. The Timer Ball's catch rate becomes higher the longer the battle lasts. So, waste time in the battle (20-30 turns should suffice) and then throw a few Timer Balls.

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14y ago

What else can I help you with?