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Technically, not necessarily. But pretty much yes.

The strict definition of a molecule the smallest particle of a substance. If that substance is a pure elemental solid then its molecule is probably a single atom, so it's obviously not more complex than an atom. But most of the time when people say "molecule" they are referring to larger ones, which are made of two or more atoms bound together is some particular structure, which is certainly more complicated than a single atom.

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