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If big means large atomic number and naturally occurring means if the world lacked humans to make nuclear tests or deposits, then Plutonium, element 94, is the answer. Some time ago plutonium was discovered in uranium ore, therefore making it the biggest, since technetium, francium, promethium, protactinium, neptunium, and other elements with atomic numbers inside the range 1 - 94 including endpoints have been found as natural, Plutonium is the biggest. Why not Americium or above? Some people say it's Californium, 98, to be the largest but alas that has been wrong since Americium all the way to Californium are only natural with pesky rocket scientists messing with fusion. Hope that helps.

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Chris Wang

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4y ago

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