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Using Crop tool you can crop image and increase resolution. Activate Crop Tool then type dimensions and resolution in tools options bar (just below menus) in Width, Height and Resolution fields then drag over image with Crop Tool to select area and confirm on check mark in tools options bar or by pressing Enter/Return. In Photoshop CS6 after activating Crop Tool click on Unconstrained on the right side of Crop Tool icon in tools options bar and choose Size and Resolution. In Crop Image Size & Resolution dialog type dimensions and Resolution or just type Resolution, confirm on OK then use Crop Tool.

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