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You cannot dissolve thinset in place. Remove any grout with MultiMaster power tool and diamond grout blade. Remove ceramic tile with a margin trowel carefully tapped under the tile with a hammer all around. Soak the tile in cheap white vinegar for 3 days to render the thinset and grout friable. Scrape it off, and repeat for tenacious deposits. Chip loose thinset off the wall, then smooth it reasonably with a MultiMaster and rasp attachment, also using the dust vacuum attachment and a shop vacuum. Wear a dust mask and goggles for all operations.

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