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Bohr's model, while groundbreaking, could not adequately explain several phenomena, including the fine structure of spectral lines and the Zeeman effect, which involves the splitting of spectral lines in a magnetic field. Additionally, it failed to account for the behavior of multi-electron atoms and the principles of wave-particle duality, as it treated electrons as particles in fixed orbits rather than incorporating their wave-like nature. The model's reliance on quantized orbits also led to inconsistencies with the principles of quantum mechanics, necessitating the development of more advanced theories like quantum mechanics and the Schrödinger equation.

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