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The biggest and the most deadly by far is when chlorine radicals destroy ozone since the reduction in use of chlorofluorocarbons the amount of chlorine radicals being pumped into the atmosphere has decreased, but chlorine radicals cannot be destroyed by reactions unless they are with each other.

cl and o3 (chlorine and ozone)

become clo and O2 (chlorineoxide and oxygen)

clo and 03

become cl and 202 (chlorine radical and 2 oxygen)

so ozone gets destroyed a lot and the cl is free again
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