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Ayatollah is a religious rank, not a specific group of individuals at a specific time. As a result, Ayatollahs have demanded many different things at different periods of time. If the question is specifically referring to the Ayatollahs of Iran in the second half of the 20th century, those Ayatollahs were demanding increasing adherence by the government to Shiite Islamic Law.
Assuming that the question refers to Iran: The Ayatollahs demanded an Iranian Constitution guaranteeing the primacy of Islamic Law in Iranian governance and themselves as its proper interpreters. This is called "Wilayat al-Faqih" in Arabic, meaning "State of the Islamic Jurist". If the question does not refer to Iran, it is worth noting that Ayatollahs in other countries such as Iraq and Lebanon have decided to support different political factions but not actually become ruling jurists.
the religious power of the ayatollahs
blloodclaut He was elected by a "Khobregan" which is a special meeting of Ayatollahs. Ayatollah Ali Khamanei was one of the members of the Supreme Council of Ayatollahs before he was brought out as their leader.
The federalists demanded constitutional amendments
Chechen fighters took over hostages in a Moscow theater and demanded the withdrawal of Russian forces from their homeland of Chechnya
ayatollahs
Depending on the context, appropriate synonyms include demanded, asserted, and took.
Middle-class professionals demanded a voice in a government
Middle-class professionals demanded a voice in government.
The national government.
The ayatollah took over after shah of Iran lost power.