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It's a very Nice question being asked..I am trying to give my thought on it ..hope it would help you out..

In both Crystallization and drying, the solute has to be separated out from its solvent (generally water) but the difference is, in former case the solute attains a pure solid state having definite shape, pattern or in other words molecules are aligned in a particular pattern but in later case the solute is having only solid shape (not necessarily having regular pattern)

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