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Pope Saint Gregory the Great (would have been Pope Gregory the First) did not create Chant or Plainsong, but gathered it together and promoted it:
from the Saints website:
Elected 64th Pope by unanimous acclamation on 3 September 590, the first monk to be chosen. Sent Saint Augustine of Canterbury and a company of monks to evangelize England, and other missionaries to France, Spain, and Africa. Collected the melodies and plain chant so associated with him that they are now known as Gregorian Chants. One of the four great Doctors of the Latin Church. Wrote seminal works on the Mass and Divine Office, several of them dictated to his secretary, Saint Peter the Deacon.
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