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There are several capital cities in South America with populations greater than 2 million. I used the CIA World Factbook to look up the populations of capital cities in South America:

Buenos Aires, Argentina: 13.528 million (2011)

Lima, Peru: 9.13 million (2011)

Bogotá, Colombia: 8.743 million (2011)

Santiago, Chile: 6.034 million (2011)

Brasilia, Brazil: 3.813 million (2011)

Caracas, Venezuela: 3.242 million (2011)

Asunción, Paraguay: 2.139 million (2011)

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