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99.9% of an atom's mass is concentrated in the nucleus, with protons and neutrons having almost the same mass, with neutrons being slightly higher. So your question would be, 'What atom has the most protons and neutrons combined?' And that answer is Nobelium. Nobelium has 102 protons and 160 neutrons which makes it the most 'massive' atomic particle, even more so then Lawrencium which has 103 protons but only 159 neutrons.

Of course, in a few months, we could have a new, more massive element.

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