There have been 22 organizations in as many countries since WW2 calling themselves "The National Liberation Front". Coming up with an original name apparently is not as easy as it looks. The mother of them all was the Viet Cong, composed of North Vietnamese and intended for the liberation and unification of Vietnam.
It you are asking about one of the other 21, please specify.
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Viet cong
National Liberation Front is the politically correct name for the Viet Cong. A group opposed by the United States
North Vietnam aided Viet Cong or the National Liberation Front (NLF) in a guerilla war against the anti-communist. The army of the North was called People's Army of Vietnam or North Vietnamese Army.
Sandinista National Liberation Front was created in 1961.
Gorkha National Liberation Front was created in 1980.
Uganda National Liberation Front was created in 1979.
Unitary National Liberation Front ended in 1945.
National Liberation Front of Tripura was created in 1989.
National Liberation Front of Angola was created in 1954.
National Liberation Front - Greece - was created in 1941.
Ogaden National Liberation Front was created in 1984.
Spanish National Liberation Front was created in 1964.
National Liberation Front is the official name for the Vietcong.
Eelam National Democratic Liberation Front was created in 1987.
United National Liberation Front - Paraguay - was created in 1960.